I think I know where you're coming from. If the sky light is all you have going for you the as you ramp down your exposure by either lowering your ISO or upping your shutter speed, your going to start to lose detail in the shadow areas. So I'm thinking by the time you get the effect of the evening as your eye sees it your camera may not pick out the detail you desire. I don't have a lot of experience in that type of light, but that's what my experience in general tells me.
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